Francesco De Bellis
Spatiotemporal Study of Electronic and Thermal Transport in Low-Dimensional Semiconductors Using Transient Reflection Microscopy.
Rel. Francesco Bertazzi. Politecnico di Torino, Corso di laurea magistrale in Nanotechnologies For Icts (Nanotecnologie Per Le Ict), 2025
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Abstract
The efficiency of silicon-based optoelectronic devices has greatly improved due to the growing knowledge of the material, yet the increasing miniaturization and performance demand is pushing research towards fundamental physical limits. At nanometer scales, carrier mobility is degraded, recombination rates affect operation speed, and thermal management becomes a challenge. Low-dimensional semiconductors such as colloidal nanocrystal (NC) films and transition metal dichalcogenides (TMDs) are therefore investigated as promising candidates for next-generation optoelectronics. The objective of this thesis is to characterize the energy transport mechanisms in these nanomaterials and identify the factors that impact on their behavior. To simultaneously access electronic and thermal carriers with sub-micrometer spatial and nanosecond temporal resolution, we employ stroboscopic scattering microscopy (stroboSCAT).
In this pump–probe technique, a focused laser pulse generates localized excited energy carriers, while a delayed wide-field probe pulse detects refractive index perturbations, enabling direct reconstruction of diffusion profiles, lifetimes, and diffusivities
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